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• W2022676588 endingPage "191" @default.
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• W2022676588 abstract "A multispectrum nonlinear least-squares fitting technique has been applied to determine accurate zero-pressure line center positions, Lorentz self- and N2-broadening coefficients and self- and N2-induced pressure shift coefficients of transitions in the ν6 (E) perpendicular band of 12CH3D between 1035 and 1270cm−1. Seventeen high-resolution (0.002–0.006cm−1) room temperature absorption spectra recorded with two Fourier transform spectrometers (FTS) were analyzed together. Self-broadening coefficients for over 700 transitions and self-shift coefficients for more than 600 transitions were determined. Measurements of nitrogen-broadening coefficients for more than 480 transitions and nitrogen pressure induced shift coefficients for nearly 430 transitions were also made. The measurements include transitions with rotational quantum numbers as high as J″=18 and K″=15 and several forbidden transitions. The measurements were made in all six sub-bands (PP,PQ,PR,RP,RQ and RR). The measured self-broadening coefficients vary from 0.025–0.096cm−1atm−1 at 296K and the N2-broadening coefficients from 0.02 to 0.08cm−1atm−1 at 296K. Self-induced-shift coefficients range from −0.014 to +0.004cm−1atm−1 while the nitrogen-induced-shift coefficients vary from −0.013 to +0.008cm−1atm−1. Very few of the measured pressure-shift coefficients were positive, and the positive shift coefficients were mostly associated with the J″=K″ transitions in the PQ sub-bands. The off-diagonal relaxation matrix element coefficients of a number of transitions with K″=3 doublets for both self- and N2-broadening were also obtained. The results obtained with the two different broadening gases are compared and discussed. Comparisons with previous values from the literature are also made." @default.
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• W2022676588 date "2002-01-01" @default.
• W2022676588 modified "2023-10-02" @default.
• W2022676588 title "Multispectrum analysis of self- and N2-broadening, shifting and line mixing coefficients in the ν6 band of 12CH3D" @default.
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• W2022676588 doi "https://doi.org/10.1016/s0022-4073(01)00120-0" @default.
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