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- W2022688003 abstract "We derive the exact third-order polarizability of a nonlinear coated sphere. We then study the effective third-order nonlinear susceptibility ${ensuremath{chi}}_{e}^{(3)}$ (Kerr coefficient) of a composite containing such coated spheres, including the interparticle interactions within mean-field theory. We show that the coated particle structure can significantly enhance the nonlinear response of a particle near resonance. Furthermore, we show that the interparticle interaction can further increase or decrease the nonlinear resonance peak by more than one order of magnitude, depending on the particle concentration, distribution, and structure, while shifting the resonance frequencies. Therefore, the spectrum of ${ensuremath{chi}}_{e}^{(3)}$ can be sensitively tuned by varying a concentration-distribution parameter." @default.
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- W2022688003 date "1997-11-01" @default.
- W2022688003 modified "2023-09-25" @default.
- W2022688003 title "Nonlinear response of composite materials containing coated spheres: Giant enhancement due to the particle structure and distribution" @default.
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- W2022688003 doi "https://doi.org/10.1103/physrevb.56.10963" @default.
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