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- W2022702545 abstract "The electronic structure of the heterodimer AlSi is experimentally studied using anion photoelectron spectroscopy. Four low-lying electronic excited states are observed for AlSi. The electron affinity of AlSi is measured to be 1.32 (5) eV, which is lower than that of both Al2 and Si2. The electronic structure of AlSi is understood by comparing to that of the known Al2 and Al2− molecules. The ground state of AlSi is determined to be X 4Σ− with a vibrational frequency of 400 (50) cm−1. The four excited states are A 2Σ−, B 2Δ, C 2Π, and D 2Σ+ with excitation energies of 0.23, 0.67, 0.82, and 1.13 eV, respectively. The photoelectron spectra of Al2− are also presented and excited states of the Al2− anion are definitively observed. The electronic structure of AlSi is discussed and compared to that of the homonuclear dimers, Al2 and Si2." @default.
- W2022702545 created "2016-06-24" @default.
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- W2022702545 date "1997-11-15" @default.
- W2022702545 modified "2023-09-27" @default.
- W2022702545 title "Electronic structure and photoelectron spectroscopy of AlSi mixed dimer" @default.
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- W2022702545 doi "https://doi.org/10.1063/1.475116" @default.
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