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- W2022706154 abstract "Abstract The reaction Eaq-+Fe2 Fe2+ was investigated by competition with the reaction Eaq-+H+ H. In acid solutions of alcohol, G(H2) was reduced very efficiently by FeIII. K 1 k 2 was determineed in HClO4 and H2SO4 and it was found to depend on the form of FeIII ion in solution. At pH 1·8, k 1 k 2 ≈2 in both HClO4 and H2SO4. Inclusion of this reaction in the mechanism of oxidation of Fe2+ in acid solutions (which has been generally neglected) confirms, as suggested by Schwarz(2), that Geaq - seems to be almost pH independent. It also removes the necessity of assuming the existence of H2O2+ which was proposed(4) (Pucheault et. al., Int. J. Radiat. Phys. Chem. 1969. 1, 209) in order to interpret the variation of G(FeIII) in acid air-saturated FeIII/Fe2+ solutions." @default.
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- W2022706154 date "1971-06-01" @default.
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- W2022706154 title "The role of the reaction of eaq - with FeIII in the radiation chemistry of acid aqueous solutions" @default.
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- W2022706154 doi "https://doi.org/10.1016/0020-7055(71)90004-0" @default.
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