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- W2022756887 abstract "Semiclassical techniques are used to analyze highly excited pure bending vibrational dynamics from spectra of C2H2. An analytic bifurcation approach is developed, based on critical points of a classical version of the quantum fitting Hamiltonian. At high energy four new types of anharmonic modes are born in bifurcations of the normal modes: local, orthogonal, precessional, and counter-rotator. Visual insight into their nature is obtained with the help of computer-generated three-dimensional animations. The connection between the local mode and the acetylene−vinylidene isomerization “reaction mode” is considered." @default.
- W2022756887 created "2016-06-24" @default.
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- W2022756887 date "2006-07-07" @default.
- W2022756887 modified "2023-09-23" @default.
- W2022756887 title "Bending Dynamics of Acetylene: New Modes Born in Bifurcations of Normal Modes" @default.
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- W2022756887 doi "https://doi.org/10.1021/jp057357f" @default.
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