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- W2022762721 abstract "When a diatomic molecule is photodissociated on a singlet molecular potential energy surface to give two singlet atoms, one of which is electronically excited, the atoms are left in pure angular momentum states referred to the molecular quantization axis. Transformation of such pure states to a laboratory frame of reference gives atomic wave functions that are described as coherent superpositions of states. Application of an external magnetic field to an ensemble of excited atoms causes quantum beats, or, alternately, a Hanle effect to appear in the fluorescence emitted by the atoms. Calculations show that the interference effects are observed only for certain geometrical arrangements of the electric vector of the photodissociating radiation, the external field, and the polarization direction accepted by the fluorescence detector. The expressions for the fluorescence intensity show that the phase and modulation depth of the quantum beat can be used to determine the asymmetry parameter for recoil of the photofragments." @default.
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- W2022762721 date "1986-07-01" @default.
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- W2022762721 title "Quantum beats in atomic fluorescence excited by molecular photodissociation" @default.
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- W2022762721 doi "https://doi.org/10.1063/1.451652" @default.
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