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- W2022762875 abstract "We consider simulations of dipolar systems under periodic boundary conditions in which a large sphere consisting of periodic replications of a central simulation cell is surrounded by a continuum of dielectric constant ε'. We develop a perturbation theory expressing correlation functions with ε in terms of correlation functions with ε' exactly to order N* 1 , N being the number of particles in the sample. In the thermodynamic limit, the correlation functions and internal energy density are independent of e The Kirkwood g -factor is strongly dependent on ε ' but in such a way as to make the dielectric constant independent of ε'. The dependence upon ε' of h A {r) at large r, described in paper I, is explained in terms of the perturbation series." @default.
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- W2022762875 date "1980-10-31" @default.
- W2022762875 modified "2023-10-03" @default.
- W2022762875 title "Simulation of electrostatic systems in periodic boundary conditions. II. Equivalence of boundary conditions" @default.
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- W2022762875 doi "https://doi.org/10.1098/rspa.1980.0136" @default.
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