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• W2022771033 abstract "We previously demonstrated that acetonitrile (NCCH3) binds to the adjacent adatom-rest atom pair of Si(111)-7×7 through a [2+2]-like cycloaddition reaction, forming a (Si)NC(Si)CH3-like surface species [Tao et al., J. Phys. Chem. B 106, 3890 (2002)]. Current investigation clearly showed that chloroacetonitrile (NCCH2Cl), propargyl chloride (HCCCH2Cl), and 3-chloropropionitrile (NCCH2CH2Cl) react with the surface via enelike reactions, concurrently involving NC/CC as well as the breakage of the CCl/CH bond. Further separation of the unsaturated bond (CC) from the CCl bond using CH2 spacers in 5-chloro-1-pentyne (CHCCH2CH2CH2Cl) would direct the reaction to a [2+2]-like cycloaddition. These experimental results clearly suggest the possibility of controlling the surface reaction pathways by tuning the organic molecular structures. This strategy can be useful in designing and fabricating functional molecular templates on Si(111)-7×7." @default.
• W2022771033 created "2016-06-24" @default.
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• W2022771033 date "2010-06-07" @default.
• W2022771033 modified "2023-10-17" @default.
• W2022771033 title "Enabling enelike reactions on Si(111)-7×7 through tuning organic molecular structures" @default.
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• W2022771033 doi "https://doi.org/10.1063/1.3407442" @default.
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