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- W2022790764 abstract "Conformationally restricted NADH peptidomimetics 4a–e, characterized by the presence of a (1,4-dihydronicotinamide)-(β-lactam) moiety, have been synthesized and used to study the Mg2+ cation-promoted asymmetric reduction of alkyl aroylformates in acetonitrile. Increasing the bulkiness of peripheral substituents at the nitrogen atom of the β-lactam ring, at the 1,4-dihydronicotinamide moiety, or at the aroylformate ester group, was found to cause weak but clearly detectable variations of the enantiomeric excess of the reaction. A rational for these observations was consistent with a chelated NADH/Mg2+/ArCOCO2R3 ternary complex model, according to DFT calculations computed at a B3LYP/6-31G∗ theory level." @default.
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- W2022790764 date "2010-04-01" @default.
- W2022790764 modified "2023-09-25" @default.
- W2022790764 title "Stereomodulating effect of remote groups on the NADH-mimetic reduction of alkyl aroylformates with 1,4-dihydronicotinamide-β-lactam amides" @default.
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- W2022790764 doi "https://doi.org/10.1016/j.tet.2010.02.085" @default.
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