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• W2022791276 abstract "The major hurdle that retards the practical application of nanostructured silicon anode in rechargeable Li-ion batteries is the capacity retention during lithiation/delithiation processes, especially at high current rate (e.g., &gt;5 C). Since fast Li transport in the electrode is the essential of high-rate capability, the rate-limiting step exists during Li transport process and needs to be determined. We here investigate Li transport properties of Si thin film anode by first-principles calculation and find that high intrinsic energy barrier (0.88 eV) of Li surface intercalation retards fast Li transport. However, this energy barrier can be efficiently reduced by surface modification, e.g., P or Al doping. The present results should shed light on designing Si anode of Li-ion batteries with high-rate capability." @default.
• W2022791276 created "2016-06-24" @default.
• W2022791276 creator A5013240931 @default.
• W2022791276 creator A5019696322 @default.
• W2022791276 creator A5049506458 @default.
• W2022791276 creator A5082857859 @default.
• W2022791276 date "2010-07-15" @default.
• W2022791276 modified "2023-10-16" @default.
• W2022791276 title "Lithium transport at silicon thin film: Barrier for high-rate capability anode" @default.
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• W2022791276 doi "https://doi.org/10.1063/1.3462998" @default.
• W2022791276 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/20649344" @default.
• W2022791276 hasPublicationYear "2010" @default.
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