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• W2022798283 abstract "We present a density-functional theory of nonuniform fluids composed of polyatomic species. It is derived from Wertheim’s first-order perturbation theory of polymerization by taking the limit of complete association. In the case of the uniform fluid, an explicit expression of the complete angle-dependent pair distribution function is obtained which shows that the theory yields nontrivial results for the intermolecular structure. However, features of the long-wavelength structure, such as the existence of an orientational order, are not described. Illustrative applications of the theory are given in the case of diatomic and linear tetra-atomic molecules formed by tangent hard spheres of the same diameter." @default.
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• W2022798283 date "1992-12-15" @default.
• W2022798283 modified "2023-10-16" @default.
• W2022798283 title "A perturbation density‐functional theory for polyatomic fluids. I. Rigid molecules" @default.
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• W2022798283 doi "https://doi.org/10.1063/1.463298" @default.
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