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• W2022832218 abstract "Abstract Chemisorbed films of ethyltrichlorosilane (ETS) at the glass/air interface are studied by IR-excitation sum-frequency (SF) spectroscopy. Using two independently tunable infrared pulses in combination with a visible upconversion pulse for the SF-probing process, a time-resolved vibrational spectroscopy is accomplished for the molecular monolayer at the dielectric surface. Rapid energy transfer in the CH-stretching region is observed with a time constant of 1.5±1 ps. The population relaxation of the CH 3 -stretching modes is found to be bimodal with a decay time of T 1 =4.5±1 ps, while the ground state is re-populated rather slowly with 130±50 ps." @default.
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• W2022832218 date "1999-09-01" @default.
• W2022832218 modified "2023-09-25" @default.
• W2022832218 title "Vibrational energy transfer of chemisorbed ethyltrichlorosilane at the glass/air interface" @default.
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• W2022832218 doi "https://doi.org/10.1016/s0009-2614(99)00801-5" @default.
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