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- W2022832880 abstract "The IR absorption coefficient for diatomic impurities dissolved in liquid solutions is calculated from a 3D model Hamiltonian. The liquid atoms surrounding the impurity form a cage that hinders strongly the molecular rotation reducing it to a librational motion. The coupling between the collective motion of the liquid and the impurity-librational motion generates the libron–phonon interaction. The shifts and broadenings of the IR spectral lines are calculated on the basis of linear response theory with a proper connected diagram analysis. Recent experimental IR measurements for CO and ClF in liquid argon are analyzed in terms of the present theory and the strength of the libron–phonon coupling for such systems is reported." @default.
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- W2022832880 title "The libron–phonon coupling and the IR absorption spectra of diatomic molecules in a simple liquid" @default.
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- W2022832880 doi "https://doi.org/10.1063/1.448409" @default.
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