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• W2022845053 abstract "The conversion of nitrous oxide in a positive pulsed corona discharge (PPCD) was studied using two stainless-steel corona reactors with the inner high-voltage electrode made of metal wire (0.3 mm in diameter). The length of the active zone was 0.75 m (reactor R1) or 0.45 m (reactor R2). In the experiments with 5% of oxygen (reactor R1), the overall conversion of N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O (to oxygen, nitrogen, and NO <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> ) considerably decreased, which was about 50% smaller than that in argon alone under the same conditions. The presence of a small amount of oxygen in the gas, containing N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O, allowed us to carry out the process using a considerably lower initial concentration of nitrous oxide. For the initial N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O concentration below 1%, it was observed that the corona discharge is not stable and changes into a spark discharge. When the N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O conversion was carried out in argon and oxygen (5% by volume), the conversion of N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O to NO <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> was 11.7% for the initial N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O concentration of 2%. The influence of oxygen in Ar + N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O (10%) on the overall conversion and conversion of N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O to NO <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> was also investigated. The increase of oxygen concentration from 5% to 45% resulted in a decrease of the overall N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O conversion and its conversion to NO <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> . PPCD could have been unstable and changed into a spark discharge when the N <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> O concentration was low." @default.
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• W2022845053 date "2009-06-01" @default.
• W2022845053 modified "2023-09-26" @default.
• W2022845053 title "Conversion of Nitrous Oxide by Positive Pulsed Corona Discharge" @default.
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• W2022845053 doi "https://doi.org/10.1109/tps.2009.2018261" @default.
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