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- W2022871528 abstract "The application of supercritical temperatures and pressures in the isomerization of n-butane is a means to avoid deactivation of the catalyst by coke and to enhance the throughputs. However, catalysts consisting of unpromoted sulfated zirconia are not sufficiently active to attain equilibrium conversions of n-butane. Through impregnation of iron salts on sulfated zirconium hydroxide, we produced catalysts containing 1 wt % iron with strongly enhanced activity. In pelletized form, these catalysts enabled the processing of n-butane at conversions close to thermodynamic equilibrium. At the preferred reaction temperature of 488 K, the yield of isobutane amounted to 43%. Catalysts manufactured by extrusion were considerably less active." @default.
- W2022871528 created "2016-06-24" @default.
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- W2022871528 date "2005-02-19" @default.
- W2022871528 modified "2023-09-27" @default.
- W2022871528 title "Approaching Equilibrium Conversion in the Isomerization of Supercritical <i>n</i>-Butane by Using Sulfated Zirconia Catalysts Promoted with Iron" @default.
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- W2022871528 doi "https://doi.org/10.1021/ie049137e" @default.
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