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- W2022962816 abstract "We present a comparative study of the charge-ordered states in orthorhombic and monoclinic forms of $ensuremath{theta}ensuremath{-}(mathrm{B}mathrm{E}mathrm{D}mathrm{T}ensuremath{-}mathrm{T}mathrm{T}mathrm{F}{)}_{2}{mathrm{TlZn}(mathrm{SCN})}_{4}$ $[mathrm{B}mathrm{E}mathrm{D}mathrm{T}ensuremath{-}mathrm{T}mathrm{T}mathrm{F}=mathrm{bis}(mathrm{ethylenedithiolo})$ tetrathiafulvalene] by means of vibrational spectroscopy with the aid of electrical resistivity and x-ray diffraction experiments. Theoretical consideration is performed for the splitting of the vibronic modes of the Raman-active $mathrm{C}=mathrm{C}$ stretching of BEDT-TTF. Based on the assignment and factor group analysis of the vibronic modes, we examined the charge-ordering pattern. The orthorhombic form provides a horizontal stripe of the localized holes, which is the same result as in the isostructural $ensuremath{theta}ensuremath{-}(mathrm{B}mathrm{E}mathrm{D}mathrm{T}ensuremath{-}mathrm{T}mathrm{T}mathrm{F}{)}_{2}{mathrm{RbZn}(mathrm{SCN})}_{4}.$ The insulator-to-insulator phase transition of the monoclinic form has been shown to be accompanied by charge ordering. In contrast to the orthorhombic form, the charge-ordering pattern is a diagonal stripe. An unusual nonmetallic state in the high-temperature phase is discussed based on the line shape of the Raman spectrum." @default.
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- W2022962816 date "2004-02-27" @default.
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- W2022962816 title "Charge-ordering transition in orthorhombic and monoclinic single-crystals of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>θ</mml:mi><mml:mo>−</mml:mo><mml:mo>(</mml:mo><mml:mi mathvariant=normal>B</mml:mi><mml:mi mathvariant=normal>E</mml:mi><mml:mi mathvariant=normal>D</mml:mi><mml:mi mathvariant=normal>T</mml:mi><mml:mo>−</mml:mo><mml:mi mathvariant=normal>T</mml:mi><mml:mi mathvariant=normal>T</mml:mi><mml:mi mathvariant=normal>F</mml:mi><mml…" @default.
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