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• W2022969228 abstract "The formation of a three-dimensional assembly of gold nanoparticles driven by host−guest interactions is described. Assembly is achieved via host−guest interactions between cyclodextrin-modified gold nanoparticles which associate with the adamantane unit of a redox active metal complex [Os(CAIPA)3](ClO4)2, where CAIPA is 2-(4-carboxyphenyl)imidazo[4,5-f][1,10]-phenanthroline-1-adamantylamine. The electrochemical properties of thin films formed on glassy carbon electrodes have been probed using cyclic voltammetry. In aqueous LiClO4, the homogeneous charge transport diffusion coefficient, DCT, is (8.4 ± 0.4) × 10−9 cm2 s−1 for both oxidation and reduction of the osmium complexes. Significantly, this charge transport rate is significantly larger than that obtained for a solid deposit of [Os(CAIPA)3](ClO4)2 alone where DCT is 2.3 × 10−10 cm2 s−1. The higher DCT value observed for the nanoparticle arrays suggests that the incorporated nanoparticles facilitate electron transfer between the bound osmium centers." @default.
• W2022969228 created "2016-06-24" @default.
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• W2022969228 date "2009-11-23" @default.
• W2022969228 modified "2023-09-25" @default.
• W2022969228 title "Host−Guest Directed Assembly of Gold Nanoparticle Arrays" @default.
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• W2022969228 doi "https://doi.org/10.1021/la902258s" @default.
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