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- W2022972041 abstract "Efficient excited‐state proton transfer in neutral acid–base clusters α‐naphthol⋅Bn has been detected and studied by a combination of laser spectroscopic techniques (resonant two‐photon ionization, fluorescence excitation, and emission spectroscopy). S1 state proton transfer was observed for B=NH3 and n≥4, as evidenced by several criteria: (a) large red shift and substantial broadening of the R2PI spectra of the n≥4 clusters relative to those of the bare α‐naphthol and smaller clusters; (b) very large Stokes shift (∼8000 cm−1) of the emission spectra of the n≥4 clusters; (c) complete broadening of the fluorescence emission band for the n≥4 clusters; and (d) a striking similarity of the emission band position and width of the latter spectra to the emission spectrum of the α‐naphtholate anion in basic aqueous solution. No proton‐transfer reaction was observed for small solvent clusters with B=NH3 and n≤3, nor for any of the pair complexes studied, which involve a single base partner [B=triethylamine, 3‐dime..." @default.
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- W2022972041 date "1988-04-01" @default.
- W2022972041 modified "2023-09-25" @default.
- W2022972041 title "Proton transfer in neutral gas‐phase clusters: α‐Naphthol⋅(NH3)n" @default.
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