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- W2023017318 abstract "Abstract There is a general question within the theory of optical basicity, which is why basicities determined by probe cations (typically Tl + and Pb 2+ ) fail to lie on the ‘theoretical’ curve linking the average basicity to glass composition. An explanation for this discrepancy is presented here, based in part on the ‘two-site’ model of Kamitsos et al. and on a dynamic site model which assumes that mobile ions (Li + , Na + , etc.) create their own sites lying along the pathways for ion migration. The experimental spread in optical basicities is attributed to this dynamic structure, and the ‘hole-digging’ capabilities of both host and probe cations. Mobile ions in singly-occupied ‘double sites’ are in relatively shallow energy wells (the L-sites), while those in doubly-occupied double sites are in relatively deep energy wells (the H-sites). Probe cations enter both H- and L-sites when their motions become coupled to those of the host cations." @default.
- W2023017318 created "2016-06-24" @default.
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- W2023017318 date "1997-12-01" @default.
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- W2023017318 title "Optical basicities and structural dynamics in glassy materials" @default.
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- W2023017318 doi "https://doi.org/10.1016/s0022-3093(97)90095-8" @default.
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