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• W2023112150 startingPage "2681" @default.
• W2023112150 abstract "The utilization of tetrahedral pre-formed coordination compounds {M(C2O4)4}4− (M = ZrIV, UIV; C2O42− = oxalate) permitted the efficient construction of rare examples of heteronuclear supramolecular nano-porous architectures. A series of metal–organic coordination frameworks prepared by association of these building units with either Mn2+, Cd2+, or Mg2+ have been structurally characterized and are described. Their 3-D chemical scaffold is based on the primary tetrahedral building unit but their pore sizes and topologies could be varied through the M2+ metal ion involved in the assembling process, and the anionic tetrahedral moiety. These structures display channels with apertures up to 12 Å × 8 Å which are emptied of solvates at mild temperatures without affecting the chemical scaffold, the integrity of which is maintained up to 250–300 °C. A certain degree of flexibility of the coordination polymers upon guest release is suggested by the temperature dependence of the powder X-ray patterns and N2 sorption experiments, but reversible and selective sorption of small molecules has been observed substantiating that these open-frameworks behave like sponges." @default.
• W2023112150 created "2016-06-24" @default.
• W2023112150 creator A5001953195 @default.
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• W2023112150 date "2005-01-01" @default.
• W2023112150 modified "2023-10-16" @default.
• W2023112150 title "Structural and zeolitic features of a series of heterometallic supramolecular porous architectures based on tetrahedral {M(C2O4)4}4– primary building units" @default.
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• W2023112150 doi "https://doi.org/10.1039/b503964a" @default.
• W2023112150 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16075106" @default.
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