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- W2023113463 abstract "Succinic 1, o-phthalic 2 and oxalic 3 acid diamides (acetonitrile-d3 solutions) as well as their perchlorates were studied by proton magnetic resonance and infrared spectroscopy. With compounds 1 and 2 the protons are added to the N atoms but no intramolecular symmetrical N+H … N ⇌ N … H+N hydrogen bonds are formed. The NH+ groups build up intramolecular asymmetrical N+H … OCN ⇌ N … HOC+N hydrogen bonds. A double-minimum energy surface is present in these intramolecular bonds. They are easily polarizable. Hydrogen-bonded N+H groups are in equilibrium with non-hydrogen-bonded N+H groupgs. With the perchlorate of oxalic acid diamide 3, the protons are added to the O atoms of carbonyl groups. Most of the O+H groups formed interact only weakly with their environment. However, a few groups form intermolecular structurally symmetrical easily polarizable O+H … O ⇌ O … H+O hydrogen bonds." @default.
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- W2023113463 date "1979-02-01" @default.
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- W2023113463 title "Intramolecular easily polarizable hydrogen bonds in diamides of succinic and o-phthalic acid" @default.
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