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- W2023113719 abstract "Polymeric pseudocrown ether networks were formed in situ by the photopolymerization of poly(ethylene glycol) diacrylate (PEGDA)/transition metal complexes. The metal−monomer complex led to a near circular conformation of the monomer in which the two reactive end groups are brought into close proximity; thus, the probability of intramolecular cyclization (i.e., pseudocrown ether formation) is increased. Complexes of cobalt(II), nickel(II), zinc(II), cadmium(II), chromium(III), copper(II), neodymium(III), and lithium were characterized using FTIR and UV−vis spectroscopy. Metal−monomer interactions were characterized and the importance of coordinated water and anions was elucidated. A novel technique of replacing coordinated waters by monomeric ether oxygens was discovered. Pseudocrown ether network formation was confirmed via a study of the polymerization kinetics of cobalt(II):PEGDA systems in which a decrease in autoacceleration was observed with increasing pseudocrown ether formation." @default.
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- W2023113719 date "2000-02-18" @default.
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- W2023113719 title "Characterization and Polymerization of Metal Complexes of Poly(ethylene glycol) Diacrylates and the Synthesis of Polymeric Pseudocrown Ethers" @default.
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- W2023113719 doi "https://doi.org/10.1021/cm990247z" @default.
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