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• W2023124530 abstract "We measure the chemical potential in a polymer melt with a modification of Widom’s insertion method. Our method is based on partial insertion of a testchain by controlling the interaction between the testchain and the melt by means of a control parameter. The chemical potential can be obtained from a single run in a multicanonical-like simulation over a wide range of temperatures and densities. From the chemical potential the osmotic pressure and the entropy are calculated. We study a variant of the bond fluctuation model of a polymer melt where an energy is gained when the bond vector is taken from the set (±3,0,0) lattice spacings (or permutations thereof). From extensive previous studies it is known that the model exhibits a glass-like freezing at low temperatures. We show that the configurational entropy decreases strongly when one cools the system through this transition, but it remains distinctly nonzero in the glass phase." @default.
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• W2023124530 date "1995-10-22" @default.
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• W2023124530 title "On the equation of state for thermal polymer solutions and melts" @default.
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• W2023124530 doi "https://doi.org/10.1063/1.470345" @default.
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