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- W2023129406 abstract "Synchrotron radiation allows monitoring of the changes in the (empty) conduction band optical density of states (CBODOS) in addition to the valence‐band (VB) and core‐level changes during (1) oxidation and (2) interface formation. Three stages of oxidation kinetics are determined in oxidation of Bi films. During the formation of Bi oxide, empty atomic‐like states of 6p1/2 character (occupied in Bi atomic ground state configuration) dominate the spectrum indicating an electron transfer from Bi to oxygen. This onset of 6p1/2 states in CBODOS occurs simultaneously with ∠2‐eV binding shifts of core levels and major changes in the VB. In the case of interface formation between cleavage planes of layered Bi2Te3 type of solids and Bi overlayers, experimental evidence is found for bonds of intermediate strength, supported by recent calculations as well as with values of Bi sticking coefficient. While Bi adatoms do not become chemically a part of Bi2Te3 substrate as evidenced by CBODOS, weak chemical bonding is suggested by weak charge redistribution as inferred from VB changes of the substrate." @default.
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- W2023129406 date "1977-01-01" @default.
- W2023129406 modified "2023-09-27" @default.
- W2023129406 title "Study of oxidation kinetics and interfacial bonding using final states" @default.
- W2023129406 doi "https://doi.org/10.1116/1.569215" @default.
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