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- W2023157649 abstract "A simple one-electron charge transfer model due to Mulliken is applied to alkali halide molecules to estimate the relative amount of parallel and perpendicular character in the “bundles” of unresolved electronic transitions which lead to dissociation and produce a normal or an excited alkali atom. If the bonding in the ground state is “purely ionic” and that in the excited state is “purely atomic,” the model indicates that most of the intensity will appear in perpendicular transitions. If the ionic and atomic character are mixed equally, however, the parallel transitions pre-empt all of the intensity, just as with purely covalent bonding. Even a slight amount of mixing (∼5%) is sufficient to put comparable intensity into the parallel and perpendicular transitions, in agreement with the scanty experimental evidence available. Numerical calculations are presented for the LiF molecule." @default.
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- W2023157649 title "Charge transfer model for alkali halide electronic transition strengths" @default.
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