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- W2023163942 abstract "The preparation of a new class of tricyclic models 1 based on a Friedländer reaction between chiral piperidine-2,4-diones 2 and azomethine 3 is reported. Alkylation of the lactam allowed to install various pendant arms on the chiral cyclic inducer. The so-obtained mimics 1a,d,f,g,h,k were involved in the reduction of methyl benzoylformate to furnish methyl mandelate in 4–87% ee (R). The presence of a coordinating pendant arm proved to be essential to reach optimum results in terms of enantioinduction. Asymmetric reduction of 2-benzoylpyridine with mimics 1d,f,g produced α-phenyl-2-pyridinemethanol in 30–84% ee (R)." @default.
- W2023163942 created "2016-06-24" @default.
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- W2023163942 date "2003-06-23" @default.
- W2023163942 modified "2023-09-25" @default.
- W2023163942 title "Chiral biomimetic NADH models in the benzo[b]-1,6-naphthyridine series. A novel class of stable, reactive and highly enantioselective NADH mimics" @default.
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- W2023163942 doi "https://doi.org/10.1016/s0040-4020(03)00706-3" @default.
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