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- W2023166441 abstract "The multiferroic RMn2O5 family, where R is rare-earth ion or Y, exhibits rich physics of multiferroicity which has not yet well understood. DyMn2O5 is a representative member of this family. The ferroelectric polarization of DyMn2O5 is claimed to be magnetically relevant and have more than one component. Therefore, the polarization reversal upon the sequent magnetic transitions is expected. We investigate the evolution of the ferroelectric polarization upon a partial substitution of Mn3+ by nonmagnetic Al3+ in order to tailor the Mn3+-Mn4+ interactions and then to modulate the polarization in DyMn2−x/2Alx/2O5. It is revealed that the polarization can be successfully reversed by Al-substitution via substantially suppressing the Mn3+-Mn4+ interactions, while the Dy3+-Mn4+ interactions can sustain against the substitution until a level as high as x = 0.2. In addition, the independent Dy spin ordering is shifted remarkably down to an extremely low temperature due to the Al3+ substitution. The present work unveils the possibility of tailoring the Mn3+-Mn4+ and Dy3+-Mn4+ interactions independently, and thus reversing the ferroelectric polarization." @default.
- W2023166441 created "2016-06-24" @default.
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- W2023166441 date "2014-08-07" @default.
- W2023166441 modified "2023-09-22" @default.
- W2023166441 title "Reversing ferroelectric polarization in multiferroic DyMn<sub>2</sub>O<sub>5</sub> by nonmagnetic Al substitution of Mn" @default.
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- W2023166441 doi "https://doi.org/10.1063/1.4891979" @default.
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