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- W2023222351 abstract "Abstract A modeling study of the effects of clouds on the evolution and redistribution of aerosol particles in the troposphere is presented. A two-mode, two-moment aerosol evolution model is coupled with a two-dimensional, mixed-phase, two-moment microphysics, Eulerian cloud model and a sulfate cloud chemistry model. The coupled model is used to simulate evolution of a convective cloud with different assumptions about the initial chemical and aerosol fields. In the simulations, SO2 is convectively transported to the mid- to upper troposphere, where it is oxidized to gas-phase H2SO4. After cloud processing, cloud condensation nuclei (CCN) particles are removed by precipitation and graupel to form a CCN-depleted region above cloud top and in the cold and humidified cloud outflow region. These conditions are favorable for binary homogeneous nucleation of ultrafine sulfuric acid particles to take place. The new particle formation in the mid- and upper troposphere interacts with cloud processing and transport ..." @default.
- W2023222351 created "2016-06-24" @default.
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- W2023222351 date "1997-10-01" @default.
- W2023222351 modified "2023-09-26" @default.
- W2023222351 title "The effects of clouds on aerosol and chemical species production and distribution: 2. Chemistry model description and sensitivity analysis" @default.
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- W2023222351 doi "https://doi.org/10.1029/97jd00775" @default.
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