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• W2023248837 abstract "Low-frequency (terahertz) motions that play an important part in reactive processes in condensed phases are directly probed, following an optical excitation. A voltage-biased semiconductor wafer, excited with a 70 femtosecond laser pulse, is employed as a source for intense terahertz pulses, which are used as the probe arm of a pump-probe experiment. Difficulties in using terahertz probe pulses are discussed. We then demonstrate the method with two examples. In the first, a terahertz signal is shown to follow the solvent response to charge transfer in betaine. In the second example, relaxation of sapphire lattice phonons, excited impulsively by a 405 nm pulse, is observed." @default.
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• W2023248837 date "1997-08-01" @default.
• W2023248837 modified "2023-10-18" @default.
• W2023248837 title "Femtosecond far-infrared pump-probe spectroscopy: A new tool for studying low-frequency vibrational dynamics in molecular condensed phases" @default.
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• W2023248837 doi "https://doi.org/10.1016/s0009-2614(97)00705-7" @default.
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