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- W2023262439 abstract "The incorporation of ${mathrm{Br}}^{ensuremath{-}}$ ions in $ensuremath{beta}ensuremath{-}mathrm{A}mathrm{g}mathrm{I}$ leads to an anomalously large increase in the ionic conductivity (${ensuremath{sigma}}_{{mathrm{Ag}}^{+}}$) and hence in the self-diffusion coefficient of ${mathrm{Ag}}^{+}$ ions (${D}_{{mathrm{Ag}}^{+}}$) as well as a substantial decrease in the first-order ($ensuremath{beta}ensuremath{-}ensuremath{alpha}$) phase-transition temperature (${T}_{c}$). The effect of substitution is found to be qualitatively analogous to that of pressure ($P$), and is attributed to purely elastic displacement (lattice distortion) caused by the wrong size of the substituent (${r}_{{mathrm{Br}}^{ensuremath{-}}}<{r}_{{mathrm{I}}^{ensuremath{-}}}$). It is concluded that the order-disorder transition is essentially driven by a critical concentration of Frenkel defects (${n}_{mathrm{ci}}$) beyond which the hexagonal $ensuremath{beta}ensuremath{-}mathrm{A}mathrm{g}mathrm{I}$ becomes unstable and transforms to disordered bcc $ensuremath{alpha}ensuremath{-}mathrm{A}mathrm{g}mathrm{I}$, a behavior consistent with the theory of Rice, Strassler, and Toombs of phase transitions to superionic conductors." @default.
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- W2023262439 date "1981-06-15" @default.
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- W2023262439 title "Phase transition and the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mi mathvariant=normal>Ag</mml:mi></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math>-ion diffusion in AgI: Effect of homovalent<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mi mathvariant=normal>Br</mml:mi></mml:mrow><mml:mrow><mml:mo>−</mml:mo></mml:mrow></mml:msup…" @default.
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- W2023262439 doi "https://doi.org/10.1103/physrevb.23.6417" @default.
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