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- W2023274908 abstract "An alternative mechanism is demonstrated to bring about light-induced kinetic effects in gases without the necessity of a state-dependent collision cross section. This is achieved by velocity-selective optical excitation followed by collisional deexcitation in the subsequent collision. This process may be termed velocity-selective heating and gives rise to an enhanced transport coefficient for a selected velocity class. A mean-free-path description of this phenomenon is given for the case of momentum transport in a one-component gas. For nonuniform illumination, a shear stress is found to result, which gives rise to light-induced viscous flow. Experimentally this effect is demonstrated for ${mathrm{CH}}_{3}$F, ${mathrm{CD}}_{3}$F, ${mathrm{CO}}_{2}$, and ${mathrm{C}}_{2}$${mathrm{H}}_{4}$, rovibrationally excited by a ${mathrm{CO}}_{2}$ laser. It is shown that the magnitude of the effect is determined by the rotational energy transfer. It can be of either sign (velocity-selective heating or cooling), depending on R- or P-branch excitation, and it can easily overwhelm the contribution to light-induced viscous flow arising from a state-dependent collision cross section." @default.
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- W2023274908 date "1991-06-01" @default.
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- W2023274908 title "Light-induced viscous flow originating from velocity-selective heating or cooling" @default.
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- W2023274908 doi "https://doi.org/10.1103/physreva.43.6135" @default.
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