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• W2023276432 abstract "The tetramers of the group 11 (I) halides, M(4)X(4) (M = Cu, Ag, or Au; X = F, Cl, Br, or I), and corresponding group 11 (I) phosphanes, chloride and bromide (XMPH(3))(4) (X = Cl or Br), are investigated by the density functional theory. All coinage metal(I) halide tetramers adopt squarelike ring structures with an out-of-plane distorted (butterfly) D(2d) symmetry. These structures are much lower in energy than the more compact cubelike T(d) arrangements, which maximize dipole-dipole interactions and more closely resemble the solid-state structures of the copper and silver halides. Phosphine coordination completely changes the structures of these M(4)X(4) clusters. The copper(I) and silver(I) phosphane chloride and bromide tetramers adopt a heterocubane structure, slightly preferred over a step (ladder-type)-cluster structure well-known in the coordination chemistry of such compounds. In stark contrast, gold(I) phosphane chloride and bromide tetramers prefer assemblies of linear XAuPH(3) units with direct gold-gold contacts, resulting in a square planar, centered trigonal planar, or tetrahedral gold core." @default.
• W2023276432 created "2016-06-24" @default.
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• W2023276432 date "2004-09-14" @default.
• W2023276432 modified "2023-10-13" @default.
• W2023276432 title "A Comparison of Structure and Stability between the Group 11 Halide Tetramers M₄X₄ (M = Cu, Ag, or Au; X = F, Cl, Br, or I) and the Group 11 Chloride and Bromide Phosphanes (XMPH₃)₄" @default.
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• W2023276432 doi "https://doi.org/10.1021/ic0492744" @default.
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