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• W2023279498 abstract "The electric field of a light wave accumulates a π phase shift as it passes through a focus. We show here how this effect, known as the Gouy phase, may be used to control the branching ratio of a unimolecular reaction when the products are formed with different numbers of photons. We demonstrate this control method for the ionization and dissociation of vinyl chloride, using absorption of 177 and 532nm photons to induce a pair of interfering paths. Excellent agreement between the observed and calculated phase shift as a function of the axial coordinate of the laser focus indicates that fragmentation occurs via a ladder switching mechanism. The axial dependence of the modulation depth is evidence of loss of coherence at higher internal temperatures of the molecule." @default.
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• W2023279498 date "2008-12-22" @default.
• W2023279498 modified "2023-10-17" @default.
• W2023279498 title "Contribution of the Gouy phase to two-pathway coherent control of the photoionization and photodissociation of vinyl chloride" @default.
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• W2023279498 doi "https://doi.org/10.1063/1.3040269" @default.
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• W2023279498 hasPublicationYear "2008" @default.
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