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• W2023302586 abstract "This study is devoted to developing amphiphilic, biodegradable, Y‐shaped block polymers, which can self‐assemble to form nanoparticles, as a glucose‐sensitive drug carrier. Y‐shaped poly(ethylene glycol)‐ block ‐[poly(lactic acid)‐ block ‐poly (2‐phenylborate esters‐1,3‐dioxane‐5‐methyl) methylacrylate)] 2 (MPEG‐(PLA‐ block ‐PPBDMMA) 2 ) polymers are constructed via a combination of ring‐opening polymerization (ROP) and atom transfer radical polymerization (ATRP) with MPEG‐(OH) 2 , having double initiation endings, as starting material. These Y‐shaped block polymers can disperse in an aqueous medium and self‐assemble into micellar aggregates with a spherical core–shell structure. Dynamic laser scattering (DLS), zeta potential measurements, and transmission electron microscopy (TEM) show the solution properties of these poly­meric micelles with or without insulin loading. Compared with MPEG‐PLA‐ block ‐PPBDMMA linear polymer, in vitro insulin release at different glucose concentrations, revealed by the fluorescence technique, shows that the studied Y‐shaped polymers have intelligent glucose‐concentration‐dependent manner of insulin release at pH 7.4 and 37 °C. The bulk swelling phenomenon of the polymeric micelles formed from the Y‐shaped polymers is detected by DLS in the process of their glucose‐responsiveness. Such a Y‐shaped glucose‐responsive polymer is a promising candidate that holds great potential in the treatment of diabetes. image" @default.
• W2023302586 created "2016-06-24" @default.
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• W2023302586 date "2014-07-17" @default.
• W2023302586 modified "2023-10-18" @default.
• W2023302586 title "Synthesis of Y-Shaped Copolymers Containing Phenylborate Ester and Biodegradable Poly(lactic acid) Blocks and Their Glucose-Sensitive Behavior for Controlled Insulin Release" @default.
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• W2023302586 doi "https://doi.org/10.1002/macp.201400195" @default.
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