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• W2023306936 abstract "The temperature dependence of NQR frequencies of halogens in ammonium hexahalotellurates(IV) has been reinvestigated in a wide range of temperature. A second-order phase transition was definitely located at 89 K for (NH4)2TeCl6, below which temperature the existence of multiplet structure was suggested The temperature of a first-order phase transition was determined for (NH4)2TeBr6 at 194 K in addition to the phase transition previously reported, which was located accurately at 212 K. The lowest-frequency line among the three 81Br resonance lines observed below 194 K exhibited a positive temperature coefficient whereas the remaining two lines showed normal negative temperature coefficients. Except for the highest-frequency v1 and v2 lines, the all four 127I lines observed for (NH4)2TeI6 showed anomalous temperature dependences. These temperature dependences could be interpreted by considering that the Te-I…H type hydrogen bonds partially break due to the thermal activation of the motion of ammonium ions in crystals. A phase transition was located at 449 K by means of differential thermal analysis." @default.
• W2023306936 created "2016-06-24" @default.
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• W2023306936 date "1989-01-01" @default.
• W2023306936 modified "2023-09-27" @default.
• W2023306936 title "Temperature dependence studies of NQR frequencies of halogens and also of quadrupolar relaxation times of chlorine nuclei in ammonium hexahalotellurates(IV)" @default.
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• W2023306936 doi "https://doi.org/10.1002/bbpc.19890930104" @default.
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