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- W2023349437 abstract "Abstract The resonant photodissociation of (CH 3 I) n + cluster ions ( n = 1–5) was studied in a crossed molecular-electron-laser beam apparatus. These results were complemented by a study of the ionization/dissociation as a function of variable energy electron ionization (EI). The fragmentation that first appears as the EI energy is raised is loss of CH 3 . This channel is particularly strong for n = 3. The lower energy dissociation of neutral I, on the other hand, is essentially quenched for cluster sizes of n > 2. Intermolecular dissociation (evaporation) of CH 3 I was evident, but was not extensive, based on a minor sensitivity of the cluster ion distribution to EI energy. The photodissociation of (CH 3 I) n + resulted in different dissociation behavior than for EI. Resonant excitation of monomer CH 3 I + to the predissociative A electronic state gave only I + CH 3 + . A state excitation of the cluster ions, on the other hand, resulted only in intermolecular dissociation. The photoexcitation cross-sections for the A 2 E 1/2 ← X 2 E 1/2 transition are presented as a function of cluster size n . A two-photon dissociation channel is also identified and the crosssections and dissociation products are reported. Finally, the frequency resolved photofragment excitation spectra of CH 3 I + and (CH 3 I) 2 + are compared." @default.
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- W2023349437 date "1996-12-01" @default.
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- W2023349437 title "Spectroscopy and photodissociation of size-selected (CH3I)n+ cluster ions" @default.
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- W2023349437 doi "https://doi.org/10.1016/s0168-1176(96)04446-1" @default.
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