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- W2023408241 abstract "We present two-photon excitation spectra for thulium III in the elpasolite Cs2NaYCl6:Tm. 37 out of the total of 40 crystal-field (CF) levels have been assigned, with the aid of a one-electron CF Hamiltonian, representing the most extensive data set so far reported for Tm III at a cubic site. Deviations from the predictions of the one-electron CF model are unusually large, the effective fourth-rank CF parameter being 60% larger for the singlet states than for the triplet states. This is discussed in terms of a spin-polarized covalency that is more pronounced in the singlet states of the metal ion." @default.
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- W2023408241 date "2001-08-02" @default.
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- W2023408241 title "Evidence for a spin-correlated crystal field - two-photon spectroscopy of thuliumIIIin the elpasolite Cs2NaYCl6:Tm" @default.
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- W2023408241 doi "https://doi.org/10.1088/0953-8984/13/33/320" @default.
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