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• W2023415061 abstract "Heat capacities of MnxFe3−xO4 with the composition x = 1.0, 1.5, and 2.0 were measured from 200 to 740 K. λ-type heat capacity anomalies due to the ferri-paramagnetic transition were observed for all the compositions. The transition temperatures were 577, 471, and 385 K for the composition x = 1.0, 1.5 and 2.0, respectively, which are in good agreement with the results of magnetic measurements. The difference in heat capacities between the different samples was small except for the temperature range of the transition. The magnetic contribution to the observed heat capacity was obtained by assuming that the heat capacity can be expressed by the sum of the lattice heat capacity Cv (l), the dilation contribution C(d), and the magnetic contribution C(m). Entropy changes due to the transition were obtained from C(m) as 55.5, 50.7 and 49.2 J K−1 mole−1 for the composition x = 1.0, 1.5, and 2.0, respectively. The entropy changes were also calculated by assuming the randomization of unpaired electron spins on each ion, but they were from 6 to 10 J K−1 mole−1 smaller than the observed ones. The difference between the experimental and the calculated values is roughly explained by taking into account the cation exchange reaction between the tetrahedral and the octahedral sites in the spinel structure." @default.
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• W2023415061 date "1981-01-01" @default.
• W2023415061 modified "2023-09-26" @default.
• W2023415061 title "Heat capacity measurements of MnxFe3−xO4" @default.
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• W2023415061 doi "https://doi.org/10.1016/0022-4596(81)90188-2" @default.
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