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• W2023481298 abstract "Resonant two-photon ionization, IR−UV hole-burning, and resonant ion-dip infrared (RIDIR) spectroscopies have been employed along with density functional theory (DFT) calculations to assign and characterize the hydrogen-bonded topologies and structures of eight benzene−(H2O)n(CH3OH)m, cluster isomers (hereafter shortened to BWnMm) with n + m ≤ 4. The O−H stretch infrared fundamentals are used to determine the H-bonding topology of the clusters. However, in several cases, the O−H stretch spectrum leaves an ambiguity regarding the position of the methanols within the structure. In these cases, the methyl CH stretch region serves as a secondary probe capable of distinguishing among the various possibilities. For n + m = 2, a single BWM isomer is observed with OH stretch fundamentals at 3508, 3606, and 3718 cm-1. A comparison of the methyl CH stretch transitions of BWM and BM2 reveals that the methanol in BWM accepts a H-bond from water and forms a π H-bond with benzene. The n + m = 3 results show the subtle ..." @default.
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• W2023481298 date "1999-01-01" @default.
• W2023481298 modified "2023-09-26" @default.
• W2023481298 title "Resonant Ion-Dip Infrared Spectroscopy of Ternary Benzene−(Water)<i>_n</i>(Methanol)<i>_m</i> Hydrogen-Bonded Clusters" @default.
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• W2023481298 doi "https://doi.org/10.1021/jp983630k" @default.
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