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• W2023493534 abstract "The pyrolysis of methane in shock waves was studied using TOF mass spectrometry, IR laser absorption, and laser schlieren techniques. The experiments spanned the temperature range 2000o–2700oK and the pressure range 20–160 kPa. The results indicate that ethylene and acetylene are formed as methane disappears. Computer simulations showed that a quantitative account for these results is afforded by mechanisms involving methyl radical chains. A set of rate constant expressions for one plausible mechanism was derived and shown also to be compatible with other studies of methane decomposition. Molecular-orbital estimates of likely reaction pathways also support this mechanism. We infer that methane combustion is accompanied by chain-reaction pyrolysis to a far greater degree than hitherto supposed." @default.
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• W2023493534 date "1975-01-01" @default.
• W2023493534 modified "2023-09-26" @default.
• W2023493534 title "Rate and mechanism of methane pyrolysis from 2000o to 2700oK" @default.
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• W2023493534 doi "https://doi.org/10.1016/s0082-0784(75)80353-5" @default.
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