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- W2023502769 abstract "The second electroviscous effect observed in charge-stabilized monodisperse colloidal suspensions as the ionic strength is lowered is tentatively predicted from a Hard-Sphere model of zero-shear viscosity η0 which depends on an effective volume fraction, eff, directly related to the HS diameter dHS defined from Russel's HS approximation. The model involves the well-known HS phase transitions (0 = 0.494 for freezing and D0 = 0.545 for melting) through the following assumptions: i) as eff < 0 (i.e. in the liquid phase) the maximum packing fraction m, involved in η0, remains close to RCP = 0.637, the random close packing, usually observed in experiments on rigid-sphere suspensions; ii) as 0 < eff < D0 (i.e. in the coexisting phase domain) m decreases continuously from RCP to D0. Model predictions are found in remarkable agreement with viscosity measurements (by C. Allain et al., 1933) on a colloidal silica suspension (for which an almost complete knowledge of physico-chemical characteristics is available), especially the variations of the zero shear viscosity vs. the actual volume fraction of particles, at ionic strength varying from 0.001 to 0.1 Mol dm-3 NaCl." @default.
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- W2023502769 title "Concentrated Colloidal Suspensions at Low Ionic Strength: A Hard-Sphere Model of Zero Shear Viscosity, Involving the Hard-Sphere Phase Transitions" @default.
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