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- W2023648767 abstract "In earlier studies on damage to model DNA systems caused by low-energy electrons, we considered electrons that attach either to cytosine's lowest π*-orbital or to a PO π*-orbital of a phosphate unit. We examined a range of electron kinetic energies (E) (e.g., representative of the Heisenberg width of the lowest π*-resonance state of cytosine), and we determined how the rates of cleavage of the sugar−phosphate C−O σ-bond depend on E and on the solvation environment. In the PO attachment study, we showed that electrons of ca. 1.0 eV could attach to form a π*-anion, which then could break either a 3‘ or 5‘ O−C σ-bond connecting the phosphate to either of two attached sugar groups. In the present study, we extend the base-attachment aspect of our work and consider electrons having kinetic energies below 1 eV attaching to thymine's lowest π*-orbital, again examining the energy and solvation dependence of the resulting rates of C−O σ-bond cleavage." @default.
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- W2023648767 date "2004-04-08" @default.
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- W2023648767 title "Damage to Model DNA Fragments by 0.25−1.0 eV Electrons Attached to a Thymine π* Orbital" @default.
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- W2023648767 doi "https://doi.org/10.1021/jp049728i" @default.
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