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• W2023667908 abstract "Abstract The effect of initial ligand concentration on the apparent rate constant of propagation of single‐electron transfer living radical polymerization (SET‐LRP) of MA in DMSO at 25 °C was examined using various lengths of Cu(0) wire as catalyst. It was determined that unlike other parameters such as initiator concentration, solvent concentration, and deactivator concentration, no simple external rate‐order for the ligand concentration could be determined. Rather, the response of the rate of SET‐LRP to initial ligand concentration is complex and is likely determined by a competition of ligand‐dependent extent of disproportionation as well as the role of ligand concentration in the surface mediated activation process. Results suggest that a minimum concentration of ligand is needed to achieve both acceptable reaction rate and reaction control, and therefore, ligand concentration must be considered in designing experimental conditions for SET‐LRP. © 2009 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 47: 5629–5638, 2009" @default.
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• W2023667908 date "2009-09-23" @default.
• W2023667908 modified "2023-10-18" @default.
• W2023667908 title "The effect of ligand on the rate of propagation of Cu(0)-wire catalyzed SET-LRP of MA in DMSO at 25 °C" @default.
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• W2023667908 doi "https://doi.org/10.1002/pola.23691" @default.
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