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• W2023678071 endingPage "114" @default.
• W2023678071 startingPage "107" @default.
• W2023678071 abstract "New measurements at 200 K, 300 K and 408 K are reported for the rate constant for the self-recombination of methyl radicals in Ar buffer gas. The 200 K measurements were made using laser flash photolysis while the 300 K and 408 K measurements were carried out at low pressures in a flow reactor. A variational RRKM calculation was performed to represent these new measurements and those previously published. The comparison between theory and experiment supports both a negative temperature dependence to the high pressure limit of recombination and a substantial positive temperature dependence to 〈ΔE〉tot, the average energy transferred in an Ar−C2H6* collision. An analytic representation of the recombination rate constant valid for all pressures where the rate constant exceeds 10−12 cm3/molecule-sec is determined over the temperature range of 200 K to 2000 K." @default.
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• W2023678071 date "1991-01-01" @default.
• W2023678071 modified "2023-10-16" @default.
• W2023678071 title "Experimental and theoretical study of the recombination reaction CH3+CH3→C2H6" @default.
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• W2023678071 doi "https://doi.org/10.1016/s0082-0784(06)80248-1" @default.
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