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- W2023687121 abstract "The dipole-quadrupole and dipole-octopole polarizabilities A and E of TiCl4, ZrCl4, and HfCl4 have been determined from collision-induced light-scattering experiments. Our respective experimental results for ∣A∣ are (165±10), (110±30), and (140±20) e2a03Eh−1, whereas ∣E∣ is determined to be (675±125), (750±200), and (670±400) e2a04Eh−1. Theory predicts values convincingly close to experiment, as A=(181.4±9.1), (167.6±8.4), and (139.8±7.0) e2a03Eh−1, and E=(−671±67), (−688±69), and (−574±57) e2a04Eh−1. In addition our quantum chemical ab initio calculations give reliable values for the dipole polarizability α, as well as for the octopole and hexadecapole moments Ω and Φ for all three substances." @default.
- W2023687121 created "2016-06-24" @default.
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- W2023687121 date "2006-03-27" @default.
- W2023687121 modified "2023-10-16" @default.
- W2023687121 title "Experimental and theoretical determination of the dipole-quadrupole and dipole-octopole polarizabilities of the group IV tetrachlorides TiCl4, ZrCl4, and HfCl4" @default.
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- W2023687121 doi "https://doi.org/10.1063/1.2181141" @default.
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