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• W2023693416 abstract "In the radiolysis of liquid water, different mechanisms for the formation of molecular hydrogen (H2) are involved at different times after the initial energy disposition. It has been suggested that the contributions of the eaq− + eaq−, H + eaq− and H + H reactions between hydrated electrons (eaq−) and hydrogen atoms in the spurs are not sufficient to account for all of the observed H2 yield (0.45 molecules/100 eV) on the microsecond time scale. Addressing the question of the origin of an unscavengeable H2 yield of 0.15 molecules/100 eV produced before spur expansion, we suggest that the dissociative capture of the so-called vibrationally-relaxing electrons by H2O molecules is a possible pathway for the formation of part of the initial H2 yield. Comparison of recent dissociative-electron-attachement H−-anion yield-distribution measurements from amorphous H2O films with the energy spectrum of vibrationally-relaxing electrons in irradiated liquid water, calculated by our Monte Carlo simulations, plays in favor of this hypothesis." @default.
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• W2023693416 date "1996-02-01" @default.
• W2023693416 modified "2023-09-30" @default.
• W2023693416 title "On the dissociative electron attachment as a potential source of molecular hydrogen in irradiated liquid water" @default.
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• W2023693416 doi "https://doi.org/10.1016/0969-806x(94)00175-j" @default.
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