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- W2023750136 abstract "The alignment dynamics of HCN, in a linear configuration, interacting with linearly polarized infrared laser pulses are studied numerically by exact (nonperturbative) solutions of the time-dependent Schrodinger equation. The alignment, with respect to the laser field polarization vector, is measured from the angular distribution of the molecule using a defined half angle ${ensuremath{theta}}_{1/2}.$ It is shown that, at intensities $mathcal{I}{=10}^{13}{mathrm{W}/mathrm{c}mathrm{m}}^{2},$ alignment can be achieved on a subpicosecond time scale with a single laser frequency, in the presence of simultaneous dipole- and polarizability-field interactions. The results are compared to those of a laser-driven rigid-rotor analytical model that is thoroughly developed. The importance of the permanent and field-induced dipole moments on the alignment process is investigated, as well as the role of vibrational excitation of the two molecular bonds." @default.
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- W2023750136 date "1999-02-01" @default.
- W2023750136 modified "2023-10-13" @default.
- W2023750136 title "Laser-induced alignment dynamics of HCN: Roles of the permanent dipole moment and the polarizability" @default.
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- W2023750136 doi "https://doi.org/10.1103/physreva.59.1382" @default.
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