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• W2023762989 abstract "X-Ray photoelectron spectroscopy (XPS) and X-ray emission spectroscopy (XES) methods were used to study the electronic structure of rhombohedral Ta4C3 and TaC0.59N0.15 compounds, as well as of several samples of the cubic TaCxN∼0.8−x system. The XPS valence band spectra and the XES Ta Lβ5 bands were derived for the rhombohedral compounds, but the Ta Lβ5, N Kα and C Kα emission bands for the cubic TaCxN∼0.8−x carbonitrides were studied and compared on a common energy scale. A strong hybridization of the Ta 5d-like and C(N) 2p-like states is characteristic of the compounds of the TaCxN∼0.8−x system studied, but the hybridization between the C 2p-like and N 2p-like states is absent. The substitution of carbon atoms for nitrogen atoms leads to increasing the metallic and ionic components and decreasing the covalent component of the chemical bonding in both systems studied. However, the metallic component is somewhat higher, but the ionic component is smaller to some degree in the rhombohedral compounds compared with those of cubic TaCxN∼0.8−x system for specimens possessing similar nitrogen-to-carbon ratios." @default.
• W2023762989 created "2016-06-24" @default.
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• W2023762989 date "2004-01-01" @default.
• W2023762989 modified "2023-10-02" @default.
• W2023762989 title "X-Ray photoelectron and emission spectra of cubic and rhombohedral tantalum carbonitrides" @default.
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• W2023762989 doi "https://doi.org/10.1016/s0925-8388(03)00472-9" @default.
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