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- W2023779778 abstract "The steady and oscillatory regions of the CO oxidation reaction on the Pd(110) surface have been determined as a function of externally controlled parameters (flow rate, CO and oxygen partial pressures, temperature) over a wide range. At constant sample temperature and flow rate, the experiments yield a characteristic cross-shaped phase diagram separating regions of monostability, bistability, and oscillatory behavior. The existence of a cross-shaped phase diagram indicates the operation of a slow feedback process, which could be traced back to the (experimentally verified) formation and retarded removal of subsurface oxygen during the reaction. The diagram reflects one of the first well-defined oscillatory systems in heterogeneous catalysis and may provide a general basis for mechanistic studies and models of oscillatory surface reactions." @default.
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- W2023779778 date "1993-06-01" @default.
- W2023779778 modified "2023-09-26" @default.
- W2023779778 title "A reactive phase diagram of CO oxidation on Pd(110): Steady and oscillatory states" @default.
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- W2023779778 doi "https://doi.org/10.1063/1.464425" @default.
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