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- W2023884395 abstract "Dissociation of well-defined ${mathrm{H}}_{3}$ Rydberg states into three ground state hydrogen atoms reveals characteristic correlation patterns in the center-of-mass motion of the three fragments. We present an extensive experimental dataset of momentum correlation maps for all lower Rydberg states of ${mathrm{H}}_{3}$ and ${mathrm{D}}_{3}$. In particular the states with principal quantum number $n=2$ feature simple correlation patterns with regular occurence of mutual affinities. Energetically higher-lying states typically show more complex patterns which are unique for each state. Quantum-chemical calculations on adiabatic potential energy surfaces of ${mathrm{H}}_{3}$ Rydberg states are presented to illuminate the likely origin of these differences. We discuss the likely dissociation mechanisms and paths which are responsible for the observed continuum correlation." @default.
- W2023884395 created "2016-06-24" @default.
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- W2023884395 date "2005-12-27" @default.
- W2023884395 modified "2023-09-27" @default.
- W2023884395 title "Experimental and quantum-chemical studies on the three-particle fragmentation of neutral triatomic hydrogen" @default.
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- W2023884395 doi "https://doi.org/10.1103/physreva.72.062506" @default.
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